| Year | Movie | Role | ||
| 1965 | The Epic That Never Was |
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| 1962 | Advise and Consent | Sen. Seabright "Seab" Cooley | ||
| 1960 | Sotto Dieci Bandiere | Adm. Russell | ||
| 1960 | Spartacus | Sempronius Gracchus | ||
| 1957 | Witness for the Prosecution | Sir Wilfrid Robarts | ||
| 1956 | Festival of Music, Vol. 1 | Host | ||
| 1953 | Young Bess | Henry VIII | ||
| 1953 | Salome | King Herod | ||
| 1953 | Hobson's Choice | Henry Horatio Hobson | ||
| 1952 | Abbott and Costello Meet Captain Kidd | Capt. Kidd | ||
| 1952 | O. Henry's Full House | Soapy, The Cop and the Anthem | ||
| 1951 | The Blue Veil | Fred K. Begley | ||
| 1951 | The Strange Door | Sire Alan de Maletroit | ||
| 1949 | The Bribe | A.J. Bealer | ||
| 1949 | The Man on the Eiffel Tower | Inspector Jules Maigret | ||
| 1948 | Arch of Triumph | Haake | ||
| 1948 | The Girl from Manhattan | The Bishop | ||
| 1948 | The Big Clock | Earl Janoth | ||
| 1947 | The Paradine Case | Judge Horfield | ||
| 1946 | Because of Him | Sheridan | ||
| 1945 | Captain Kidd | Capt. William Kidd | ||
| 1944 | The Suspect | Philip | ||
| 1944 | The Canterville Ghost | Sir Simon de Canterville/The Ghost | ||
| 1943 | This Land Is Mine | Arthur Lory | ||
| 1943 | The Man from Down Under | Jocko Wilson | ||
| 1943 | Forever and a Day | Bellamy, Dexter Pomfret's Butler | ||
| 1942 | The Tuttles of Tahiti | Jonas Tuttle | ||
| 1942 | Tales of Manhattan | Charles Smith | ||
| 1942 | Stand by for Action | Rear Adm. Stephen Thomas | ||
| 1941 | It Started With Eve | Jonathan Reynolds | ||
| 1940 | They Knew What They Wanted | Tony Patucci | ||
| 1939 | The Hunchback of Notre Dame | Quasimodo | ||
| 1939 | Jamaica Inn | Sir Humphrey Pengallan | ||
| 1938 | The Beachcomber | Ginger Ted | ||
| 1938 | Sidewalks of London | Charles Saggers | ||
| 1936 | Rembrandt | Rembrandt van Rijn | ||
| 1935 | Les Miserables | Javert | ||
| 1935 | Ruggles of Red Gap | Marmaduke Ruggles | ||
| 1935 | Mutiny on the Bounty | Capt. William Bligh | ||
| 1934 | The Barretts of Wimpole Street | Edward Moulton Barrett | ||
| 1933 | The Private Life of Henry VIII | Henry VIII | ||
| 1933 | White Woman | Horace Prin | ||
| 1932 | The Sign of the Cross | Nero | ||
| 1932 | If I Had a Million | The Clerk | ||
| 1932 | Island of Lost Souls | Dr. Moreau | ||
| 1932 | Payment Deferred | William Marble | ||
| 1932 | The Old Dark House | Sir William Porterhouse | ||
| 1932 | The Devil and the Deep | Commander Charles Storm | ||
| 1931 | Down River | Capt. Grossman | ||
| 1930 | Wolves | Capt. Job | ||
| 1929 | Piccadilly | A Night Club Hawk | ||
| Pirates: Dead Men Tell Their Tales | Captain Kidd |
| Year | Movie | Role | ||
| 1955 | The Night of the Hunter | Director | ||
| 1939 | Jamaica Inn | Producer | ||
| 1938 | Sidewalks of London | Screenwriter |
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